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The development of electrocatalytic’ systems depends in part
on the development of systems that can undergo multiple electron
transfers as well as being amenable to the fine tuning of redox
potentials through synthetic variations or other means. This is
dictated in part by the need to have systems whose redox levels
can be shifted so as to achieve a good match with those of the
desired rection and also by the need to transfer more than one
electron so as to circumvent the formation of high-energy intermediates.
These aspects have been explored in a number of applications.
Meyer2 very recently made an extensive exposition of how to
control reactivity by suitably modifying the coordination environment
around a metal ion as well as how to achieve multiple
electron transfers by coupling redox processes associated with
dimers or higher order clusters. He also pointed to the importance
of structural aspects in achieving de

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